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Contents

Foreword

Preface

Scheme of the Book, Figures, Notes, and Abbreviations

Acknowledgments

List of 42 Marcus’ Papers Closely Followed, Summarized or Abridged in Chapters 2–11 and of 10 Papers Considered in the Oral Interviews of Chapters 12 and 13

List of Marcus’ Papers Considered in the Chapters of the Book

Chapter 1Introduction

Chapter 2Foundations of the Theory, Its First Formulation

Chapter 3Extensions, Electron Transfer at Electrodes, Applications

Chapter 4Theory of Electrochemical Electron Transfer

Chapter 5Statistical Mechanical Theory of Electron Transfer, Equivalent Equilibrium Distribution, Reaction Coordinate for ET, Inverted Free Energy Effect, Interactions in Polar Media

Chapter 6Unified General Theory of Electron Transfer Reactions

Chapter 7Theory of Electron Transfer Reactions of Solvated Electrons and of Chemiluminescent Electron Transfer Reactions

Chapter 8Rate Constants, Barriers, and Brønsted Slopes, Electron Transfer at Electrodes and in Solution: Theory versus Experiment—Electrode Reactions of Organic Compounds

Chapter 9Activated-Complex Theory, Application to Electron Transfer Reactions. Marcus’ Notes on Electron Transfer, on Proton Transfer and on Electrode Kinetics

Chapter 10Unusual Activation Parameters, Electron and Nuclear Tunneling, Mechanisms of Charge Separation, Spin Exchange and Electron Transfer in Photosynthesis; Electron Transfer versus Proton Transfer at Electrodes and in Solution, Hydrogen Evolution, Quantum Effects, Classical and Semiclassical Calculations of Electron Transfer Rates

Chapter 11Mixed Reaction-Diffusion Rates, Quantum Effects in the Inverted Region, Frequency Factor in Electron Transfer: Its Role in the Highly Exothermic Regime, Highly Exothermic Electron Transfer, Electron and Proton Transfer, Nonadiabatic Processes, Quantum-like and Classical-like Coordinates, Applications to Nonadiabatic Electron Transfers

Chapter 12Entropic, Electrolyte, and Orientation Effects in Electron Transfer, Electron Transfer in Chemistry and Biology, Application of Electron Transfer to Systems of Biological Interest, Barriers for Thermal and Optical Electron Transfer in Solution, Semiclassical Model for Orientation Effects in Electron Transfer, Orientation Effects on Electron Transfer between Porphyrins

Chapter 13Dynamical Effects in Electron Transfer Reactions, Dielectric Relaxation and Intramolecular Electron Transfer, Solvent Dynamics, and Vibrational Effects in Electron Transfer