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Heterogeneous Catalysts
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Страница 1
Table of Contents
List of Tables
List of Illustrations
Guide
Pages
Heterogeneous Catalysts Advanced Design, Characterization and Applications
Heterogeneous Catalysts Advanced Design, Characterization and Applications
Страница 9
Preface
Страница 11
1 Evolution of Catalysts Design and Synthesis: From Bulk Metal Catalysts to Fine Wires and Gauzes, and that to Nanoparticle Deposits, Metal Clusters, and Single Atoms
1.1 The Cradle of Modern Heterogeneous Catalysts
1.2 The Game Changer: High‐Pressure Catalytic Reactions
1.3 Catalytic Cracking and Porous Catalysts
1.4 Miniaturization of Metal Catalysts: From Supported Catalysts to Single‐Atom Sites
1.5 Perspectives and Opportunities
References
2 Facets Engineering on Catalysts
2.1 Introduction
2.2 Mechanisms of Facets Engineering
2.3 Anisotropic Properties of Crystal Facets
2.3.1 Anisotropic Adsorption
2.3.2 Surface Electronic Structure
2.3.3 Surface Electric Field
2.4 Effects of Facets Engineering
2.4.1 Optical Properties
2.4.2 Activity and Selectivity
2.5 Outlook
References
3 Electrochemical Synthesis of Nanostructured Catalytic Thin Films
3.1 Introduction
3.2 Principle of Electrochemical Method in Fabricating Thin Film
3.2.1 Anodization
3.2.1.1 Pulse or Step Anodization
3.2.2 Cathodic Electrodeposition
3.2.2.1 Pulse Electrodeposition
3.2.3 Electrophoretic Deposition
3.2.4 Combinatory Methods Involving Electrochemical Process
3.2.4.1 Combined Electrophoretic Deposition–Anodization (CEPDA) Approach
3.3 Conclusions and Perspective
References
4 Synthesis and Design of Carbon‐Supported Highly Dispersed Metal Catalysts
4.1 Introduction
4.2 Preparation of Catalysts on New Carbon Supports
4.2.1 Catalyst on Graphene Oxide
4.2.2 Catalyst on Graphene
4.2.2.1 Graphene or rGO as Starting Material
4.2.2.2 Graphene Oxide as Precursor of Graphene‐Supported Catalyst
4.2.2.3 Graphene Derivatives: Doped Graphene and Synthetic Derivatives
4.2.3 Catalyst on Nanodiamonds and Onion‐Like Carbon
4.2.4 SACs on Carbon Nitrides and Covalent Triazine Frameworks
4.2.5 Catalyst on Carbon Material from Hydrothermal Carbonization of Biomolecules
4.3 Emerging Techniques for Carbon‐Based Catalyst Synthesis
4.3.1 Deposition of Colloidal Nanoparticles
4.3.2 Single‐Metal Atom Deposition by Wet Chemistry
4.3.3 Immobilization of Metal Clusters and SACs by Organometallic Approach
4.3.4 Chemical Vapor Deposition Techniques on Carbon Supports
4.3.5 Simultaneous Formation of Metallic Catalyst and Porous Carbon Support by Pyrolysis
4.3.6 Dry Mechanical Methods
4.3.7 Electrodeposition
4.3.8 Photodeposition
4.4 Conclusions and Outlook
References
5 Metal Cluster‐Based Catalysts
5.1 Introduction
5.2 Catalysts Made by Deposition of Clusters from the Gas Phase Under Ultrahigh Vacuum
5.3 Chemically Synthesized Metal Clusters
5.4 Catalysis Using the Chemically Synthesized Metal Clusters
5.5 Conclusion
References
6 Single‐Atom Heterogeneous Catalysts
6.1 Introduction
6.2 Concept and Advantages of SACs 6.2.1 Concept of SACs
6.2.2 Advantages of SACs 6.2.2.1 Maximum Atom Efficiency
6.2.2.2 Unique Catalytic Properties
6.2.2.3 Identification of Catalytically Active Sites
6.2.2.4 Establishment of Intrinsic Reaction Mechanisms
6.3 Synthesis of SACs
6.3.1 Physical Methods
6.3.2 Chemical Methods
6.3.2.1 Bottom‐Up Synthetic Methods
6.3.2.2 Top‐Down Synthetic Methods
6.4 Challenges and Perspective
References
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