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This work was supported by the U.S. Department of Energy (DOE) through the Los Alamos National Laboratory (LANL) operated by Triad National Security, LLC, for the National Nuclear Security Administration (NNSA) of U.S. DOE under Contract No. 89233218CNA000001, and through Lawrence Livermore National Laboratory (LLNL) under Contract DE‐AC52‐07NA27344. We thank the AGU Publications Director Dr. Jenny Lunn and Dr. Estella Atekwana of the AGU Books Editorial Board for their careful review and valuable comments. We also thank David Li of LANL for his review. This chapter is approved for public release by LANL (LA‐UR‐21‐27246) and by LLNL (LLNL‐BOOK‐824879).